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Preview of Formaldehyde Inhibition
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Summary

Formaldehyde inhibits hydrogen evolution by [FeFe]-hydrogenases by binding close to the active site, forming a short Fe−13C bond in the 2Fe subsite, and acting as a metal-hydrido mimic, preventing the formation of the transient species Hox−2(2H) and supporting a mechanism involving two consecutive proton transfer steps to the H-cluster following transfer of a second electron to the active site.

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Formaldehyde inhibits hydrogen evolution by [FeFe]-hydrogenases by binding close to the active site, forming a short Fe−13C bond in the 2Fe subsite, and acting...

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  • File Format: PDF
  • File Size: 1.64 MB
  • Pages: 9
  • Language: EN
  • Total Downloads: 68
  • Last Updated: 1 week ago

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