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Molecular Rotors.pdf

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Preview of Molecular Rotors
🔗 Source: pure.uva.nl
📊 Size: 1.28 MB
📄 Pages: 22 pages
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Summary

Fluorescent molecular rotors' fluorescence intensity increases with solvent viscosity, with single-bond and double-bond rotations proposed as nonradiative decay pathways. Steady-state and time-resolved fluorescence measurements, combined with visible-pump/mid-IR probe transient measurements and TD-DFT calculations, show that both single and double bond rotations are involved in DCDHF rotors' decay, with fluorescence quenched by rotation around the dicyanomethylene double bond in non-polar solvents and by rotation about a single bond in polar environments, leading to a dark internal charge-transfer state.

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Description

Fluorescent molecular rotors' fluorescence intensity increases with solvent viscosity, with single-bond and double-bond rotations proposed as nonradiative...

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  • File Format: PDF
  • File Size: 1.28 MB
  • Pages: 22
  • Language: EN
  • Total Downloads: 135
  • Last Updated: 1 week ago

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